eprintid: 9333 rev_number: 2 eprint_status: archive userid: 1 dir: disk0/00/00/93/33 datestamp: 2023-11-09 16:21:18 lastmod: 2023-11-09 16:21:18 status_changed: 2023-11-09 16:14:52 type: article metadata_visibility: show creators_name: Tay, W.H. creators_name: Lau, K.K. creators_name: Shariff, A.M. title: High frequency ultrasonic-assisted chemical absorption of CO2 using monoethanolamine (MEA) ispublished: pub keywords: Carbon dioxide; Irradiation; Mass transfer, Chemical absorption; CO2 absorption; Convective dynamics; Enhancement effects; Gas liquids; High frequency HF; Monoethanolamine solvent; Ultrasound irradiation, Ethanolamines note: cited By 30 abstract: The paper aimed to study the chemical absorption of CO2 in monoethanolamine solvent (MEA) using high frequency ultrasonic irradiation of 1.7 MHz. The experiment was conducted at instantaneous regime in order to study the physical enhancement effect of the ultrasound. Hence, a mathematical model is proposed to justify the enhancement effects involved in the absorption process. The parameters of the experiment included ultrasonic power, MEA concentration, temperature, and CO2 partial pressure. Results show that, a significant increase in the chemical absorption rate can be obtained by using ultrasonic power of 18 W, which is up to 60 times faster than the case without ultrasonic irradiation. Besides, the experimental data is in good agreement with the simulated data by obtaining the R2 values ranged from 0.989 to 0.997. Therefore, this study demonstrates a new technology to improve the absorption process. Besides, the enhancement for the chemical absorption using ultrasonic irradiation is believed to be dominated by the fountain formation and also the convective dynamic. In overall, ultrasonic-assisted absorption would be one of the potential alternatives for CO2 capture with its advantages of high mass transfer coefficient and compact design. © 2017 Elsevier B.V. date: 2017 publisher: Elsevier B.V. official_url: https://www.scopus.com/inward/record.uri?eid=2-s2.0-85017230551&doi=10.1016%2fj.seppur.2017.03.068&partnerID=40&md5=a543fff03b2f257e348363f3922cb621 id_number: 10.1016/j.seppur.2017.03.068 full_text_status: none publication: Separation and Purification Technology volume: 183 pagerange: 136-144 refereed: TRUE issn: 13835866 citation: Tay, W.H. and Lau, K.K. and Shariff, A.M. (2017) High frequency ultrasonic-assisted chemical absorption of CO2 using monoethanolamine (MEA). Separation and Purification Technology, 183. pp. 136-144. ISSN 13835866